| Name | Country | Years |
| Louis Goffin | Belgium | 1955–1962 |
| Maurice Iweins d'Eeckhoutte | Belgium | 1962–1970 |
| Georges Heisbourg | Luxembourg | 1971–1974 |
| Friedrich-Karl von Plehwe | West Germany | 1974–1977 |
| Edouard Longerstaey | Belgium | 1977–1985 |
| Alfred Cahen | Belgium | 1985–1989 |
| Wim van Eekelen | Netherlands | 1989–1994 |
| José Cutileiro | Portugal | 1994–1999 |
| Javier Solana | Spain | 1999–2009 |
| Arnaud Jacomet | France | 2009–2011 |
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